I also found on his site a link to the Vatican Film List which is an old list from 1995 that was comprised by the Vatican for the 100th anniversary of cinema. It included a top ten list of movies for religion, value and art. I perused through that list too and was familiar with a few.
I would imagine the movie The Way starring Martin Sheen and written, directed and starring Emilio Estevez, would be added to Mr. Graydanus's recommendations for Lent and Films. This movie came out on DVD last month to my delight! I have bought it, viewed it and have passed it around to friends from my church. If you haven't seen it yet, please do! It should be in the local libraries by now if you don't want to purchase your own copy.